Light-Induced Paramagnetism in Colloidal Ag<sup>+</Sup>-doped Cdse Nanoplatelets
| dc.authorid | SHARMA, MANOJ/0000-0002-0601-2665 | |
| dc.authorid | Demir, Hilmi Volkan/0000-0003-1793-112X | |
| dc.authorid | Delikanli, Savas/0000-0002-0613-8014 | |
| dc.authorid | Erdem, Onur/0000-0003-2212-965X | |
| dc.authorid | Najafi, Arman/0000-0002-8022-5095 | |
| dc.authorid | Murphy, Joseph/0000-0002-9947-995X | |
| dc.authorid | Pientka, James/0000-0003-3167-4246 | |
| dc.authorscopusid | 57211277081 | |
| dc.authorscopusid | 57204309965 | |
| dc.authorscopusid | 25222326900 | |
| dc.authorscopusid | 57224708752 | |
| dc.authorscopusid | 55279248600 | |
| dc.authorscopusid | 55247038400 | |
| dc.authorscopusid | 35552742000 | |
| dc.authorwosid | Kovalenko, Maksym V/B-6844-2008 | |
| dc.authorwosid | SHARMA, MANOJ/C-5325-2019 | |
| dc.authorwosid | delikanli, savas/KBR-2849-2024 | |
| dc.authorwosid | Demir, Hilmi Volkan/AAV-2194-2020 | |
| dc.authorwosid | Sharma, Manoj/I-8493-2018 | |
| dc.contributor.author | Najafi, Arman | |
| dc.contributor.author | Sharma, Manoj | |
| dc.contributor.author | Delikanli, Savas | |
| dc.contributor.author | Bhattacharya, Arinjoy | |
| dc.contributor.author | Murphy, Joseph R. | |
| dc.contributor.author | Pientka, James | |
| dc.contributor.author | Petrou, Athos | |
| dc.date.accessioned | 2024-07-05T15:21:23Z | |
| dc.date.available | 2024-07-05T15:21:23Z | |
| dc.date.issued | 2021 | |
| dc.department | Atılım University | en_US |
| dc.department-temp | [Najafi, Arman; Bhattacharya, Arinjoy; Quinn, Alexander P.; Petrou, Athos] Univ Buffalo SUNY, Dept Phys, Buffalo, NY 14260 USA; [Sharma, Manoj; Delikanli, Savas; Sharma, Ashma; Demir, Hilmi Volkan] Nanyang Technol Univ, Luminous Ctr Excellence Semicond Lighting & Displ, Sch Elect & Elect Engn, Singapore 639798, Singapore; [Sharma, Manoj; Delikanli, Savas; Sharma, Ashma; Demir, Hilmi Volkan] Nanyang Technol Univ, Div Phys & Appl Phys, Sch Phys & Math Sci, Singapore 639798, Singapore; [Sharma, Manoj; Delikanli, Savas; Erdem, Onur; Demir, Hilmi Volkan] Bilkent Univ, UNAM Inst Mat Sci & Nanotechnol, Dept Elect & Elect Engn, TR-06800 Ankara, Turkey; [Sharma, Manoj; Delikanli, Savas; Erdem, Onur; Demir, Hilmi Volkan] Bilkent Univ, UNAM Inst Mat Sci & Nanotechnol, Dept Phys, TR-06800 Ankara, Turkey; [Murphy, Joseph R.] Southeast Missouri State Univ, Dept Chem & Phys, Cape Girardeau, MO 63701 USA; [Murphy, Joseph R.; Kattel, Subash; Rice, William D.] Univ Wyoming, Dept Phys & Astron, Laramie, WY 82071 USA; [Pientka, James] St Bonaventure Univ, Dept Phys, St Bonaventure, NY 14778 USA; [Kelestemur, Yusuf; Kovalenko, Maksym, V] Swiss Fed Inst Technol, Dept Chem & Appl Biosci, CH-8093 Zurich, Switzerland; [Kelestemur, Yusuf] Atilim Univ, Dept Met & Mat Engn, TR-06830 Ankara, Turkey; [Kovalenko, Maksym, V] Empa Swiss Fed Labs Mat Sci & Technol, CH-8600 Dubendorf, Switzerland | en_US |
| dc.description | SHARMA, MANOJ/0000-0002-0601-2665; Demir, Hilmi Volkan/0000-0003-1793-112X; Delikanli, Savas/0000-0002-0613-8014; Erdem, Onur/0000-0003-2212-965X; Najafi, Arman/0000-0002-8022-5095; Murphy, Joseph/0000-0002-9947-995X; Bhattacharya, Arinjoy/0000-0002-8019-4233; Sharma, Manoj/0000-0001-5215-9740; Pientka, James/0000-0003-3167-4246 | en_US |
| dc.description.abstract | We describe a study of the magneto-optical properties of Ag+-doped CdSe colloidal nanoplatelets (NPLs) that were grown using a novel doping technique. In this work, we used magnetic circularly polarized luminescence and magnetic circular dichroism spectroscopy to study light-induced magnetism for the first time in 2D solution-processed structures doped with nominally nonmagnetic Ag+ impurities. The excitonic circular polarization (P-X) and the exciton Zeeman splitting (Delta E-Z) were recorded as a function of the magnetic field (B) and temperature (T). Both Delta E-Z and P-X have a Brillouin-function-like dependence on B and T, verifying the presence of paramagnetism in Ag+-doped CdSe NPLs. The observed light-induced magnetism is attributed to the transformation of nonmagnetic Ag+ ions into Ag2+, which have a nonzero magnetic moment. This work points to the possibility of incorporating these nanoplatelets into spintronic devices, in which light can be used to control the spin injection. | en_US |
| dc.description.sponsorship | NSF MRI Award [1726303]; Singapore National Research Foundation [NRF-NRFI2016-08, NRF-CRP14-2014-03]; Science and Engineering Research Council, Agency for Science, Technology, and Research (A*STAR) of Singapore; TUBA; European Union's Horizon 2020 research and innovation program under the Marie Sklodowska-Curie grant [798697]; Scientific Center for Optical and Electron Microscopy (ScopeM) of the Swiss Federal Institute of Technology ETHZ; Division Of Materials Research; Direct For Mathematical & Physical Scien [1726303] Funding Source: National Science Foundation; Marie Curie Actions (MSCA) [798697] Funding Source: Marie Curie Actions (MSCA) | en_US |
| dc.description.sponsorship | A.P. acknowledges support from the NSF MRI Award 1726303. M.S. and H.V.D. acknowledge the financial support from the Singapore National Research Foundation under the Programs of NRF-NRFI2016-08, NRF-CRP14-2014-03, and the Science and Engineering Research Council, Agency for Science, Technology, and Research (A*STAR) of Singapore. H.V.D. acknowledges additional financial support from the TUBA. M.V.K. and Y.K. acknowledge financial support from the European Union's Horizon 2020 research and innovation program under the Marie Sklodowska-Curie grant no. 798697. We acknowledge the support of the Scientific Center for Optical and Electron Microscopy (ScopeM) of the Swiss Federal Institute of Technology ETHZ. | en_US |
| dc.identifier.citationcount | 19 | |
| dc.identifier.doi | 10.1021/acs.jpclett.1c00398 | |
| dc.identifier.endpage | 2899 | en_US |
| dc.identifier.issn | 1948-7185 | |
| dc.identifier.issue | 11 | en_US |
| dc.identifier.pmid | 33724845 | |
| dc.identifier.scopus | 2-s2.0-85103607805 | |
| dc.identifier.startpage | 2892 | en_US |
| dc.identifier.uri | https://doi.org/10.1021/acs.jpclett.1c00398 | |
| dc.identifier.uri | https://hdl.handle.net/20.500.14411/2073 | |
| dc.identifier.volume | 12 | en_US |
| dc.identifier.wos | WOS:000635441500026 | |
| dc.identifier.wosquality | Q1 | |
| dc.language.iso | en | en_US |
| dc.publisher | Amer Chemical Soc | en_US |
| dc.relation.publicationcategory | Makale - Uluslararası Hakemli Dergi - Kurum Öğretim Elemanı | en_US |
| dc.rights | info:eu-repo/semantics/openAccess | en_US |
| dc.scopus.citedbyCount | 24 | |
| dc.subject | [No Keyword Available] | en_US |
| dc.title | Light-Induced Paramagnetism in Colloidal Ag<sup>+</Sup>-doped Cdse Nanoplatelets | en_US |
| dc.type | Article | en_US |
| dc.wos.citedbyCount | 24 | |
| dspace.entity.type | Publication |