Utilization of TRISO fuel with reactor grade plutonium in CANDU reactors

Abstract

Large quantities of plutonium have been accumulated in the nuclear waste of civilian LWRs and CANDU reactors. Reactor grade plutonium and heavy water moderator can give a good combination with respect to neutron economy. On the other hand. TRISO type fuel can withstand very high fuel burn-up levels. The paper investigates the prospects of utilization of TRISO fuel made of reactor grade plutonium in CANDU reactors. TRISO fuels particles are imbedded body-centered cubic (BCC) in a graphite matrix with a volume fraction of 68%. The fuel compacts conform to the dimensions of CANDU fuel compacts are inserted in rods with zircolay cladding. In the first phase of investigations, five new mixed fuel have been selected for CANDU reactors composed of (1) 4% RG-PuO2+ 96% ThO2; CD 6% RG-PuO2 + 94% ThO2; (3) 10% RG-PuO2+ 90% ThO2; 20% RG-PuO2+ 80% ThO2; (5) 30% RG-PuO2 + 70% ThO2. Initial reactor criticality (k(infinity,0) values) for the modes (1), (2), (3), (4) and are calculated as 1.4294, 1.5035, 1.5678, 1.6249, and 1.6535, respectively. Corresponding operation lifetimes are similar to 0.65, 1.1, 1.9.3.5, and 4.8 years and with burn ups of 30000, 60000, 100000. 200000 and 290000 MW d/tonne, respectively. The higher initial plutonium charge is the higher burn ups can be achieved. In the second phase, a graphical-numerical power flattening procedure has been applied with radially variable mixed fuel composition in the fuel bundle. Mixed fuel fractions leading to quasi-constant power production are found in the 1st, 2nd. 3rd and 4th row to be as 100% PuO2, 80/20% PuO2/ThO2, 60/40% PuO2/ThO2, and 40/60% PuO2/ThO2, respectively. Higher plutonium amount in the flattened case increases reactor operation lifetime to >8 years and the burn up to 580 000 MW d/tonne. Power flattening in the bundle leads to higher power plant factor and quasi-uniform fuel utilization, reduces thermal and material stresses, and avoids local thermal peaks. Extended burn-up grade implies drastic reduction of the nuclear waste material per unit energy output for final waste disposal. (C) 2010 Elsevier BM. All rights reserved.